385 research outputs found
Lithium Ionization by a Strong Laser Field
We study ab initio computations of the interaction of Lithium with a strong
laser field. Numerical solutions of the time-dependent fully-correlated
three-particle Schroedinger equation restricted to the one-dimensional
soft-core approximation are presented. Our results show a clear transition from
non-sequential to sequential double ionization for increasing intensities. Non
sequential double ionization is found to be sensitive to the spin configuration
of the ionized pair. This asymmetry, also found in experiments of
photoionization of Li with synchrotron radiation, shows the evidence of the
influence of the exclusion principle in the underlying rescattering mechanism
High-order harmonic generation at high laser intensities beyond the tunnel regime
We present studies of high-order harmonic generation (HHG) at laser
intensities well above saturation. We use driving laser pulses which present a
particular electron dynamics in the turn-on stage. Our results predict an
increasing on the harmonic yield, after an initial dropping, when the laser
intensity is increased. This fact contradicts the general belief of a
progressive degradation of the harmonic emission at ultrahigh intensities. We
have identified a particular set of trajectories which emerges in the turn-on
stage of these singular laser pulses, responsible of the unexpected growth on
the harmonic efficiency at this high intensity regime. Our study combines two
complementary approaches: classical analysis and full quantum mechanical
calculations resulting from the numerical integration of the 3-dimensional
time-dependent Schr\"odinger equation complemented with the time-frequency
analysis
High-order harmonic generation driven by chirped laser pulses induced by linear and non linear phenomena
We present a theoretical study of high-order harmonic generation (HHG) driven
by ultrashort optical pulses with different kind of chirps. The goal of the
present work is perform a detailed study to clarify the relevant parameters in
the chirped pulses to achieve a noticeable cut-off extensions in HHG. These
chirped pulses are generated using both linear and nonlinear dispersive
media.The description of the origin of the physical mechanisms responsible of
this extension is, however, not usually reported with enough detail in the
literature. The study of the behaviour of the harmonic cut-off with these kind
of pulses is carried out in the classical context, by the integration of the
Newton-Lorentz equation complemented with the quantum approach, based on the
integration of the time dependent Schr\"odinger equation in full dimensions
(TDSE-3D), we are able to understand the underlying physics.Comment: 13 pages, 8 figure
Carrier-wave Rabi flopping signatures in high-order harmonic generation for alkali atoms
We present the first theoretical investigation of carrier-wave Rabi flopping
in real atoms by employing numerical simulations of high-order harmonic
generation (HHG) in alkali species. Given the short HHG cutoff, related to the
low saturation intensity, we concentrate on the features of the third harmonic
of sodium (Na) and potassium (K) atoms. For pulse areas of 2 and Na atoms,
a characteristic unique peak appears, which, after analyzing the ground state
population, we correlate with the conventional Rabi flopping. On the other
hand, for larger pulse areas, carrier-wave Rabi flopping occurs, and is
associated with a more complex structure in the third harmonic. These new
characteristics observed in K atoms indicate the breakdown of the area theorem,
as was already demonstrated under similar circumstances in narrow band gap
semiconductors
Nonlinear resonance reflection from and transmission through a dense glassy system built up of oriented linear Frenkel chains: two-level models
A theoretical study of the resonance optical response of assemblies of
oriented short (as compared to an optical wavelength) linear Frenkel chains is
carried out using a two-level model. We show that both transmittivity and
reflectivity of the film may behave in a bistable fashion and analyze how the
effects found depend on the film thickness and on the inhomogeneous width of
the exciton optical transition.Comment: 26 pages, 9 figure
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